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題名 Bright and Dark Plasmon Modes in Three Nanocylinder Cluster
作者 郭光宇
Klimov, Vasily ; Guo, Guang-Yu
貢獻者 應物所
日期 2010.12
上傳時間 28-Apr-2014 17:42:36 (UTC+8)
摘要 Plasmonic excitations in a three interacting nanocylinder cluster have been investigated by both simple analytical modeling and discrete dipole approximation (DDA) calculations. In our analytical model, each cylinder is regarded as an anisotropic electric dipole with four parameters determined by fitting its optical extinction and scattering spectra to that of DDA simulation. Diagonalization of our analytical model for the three interacting dipoles reveals 10 significant plasmon modes, namely, 5 bright modes and 5 dark eigen-modes. Because of rather long-range longitudinal plasmon coupling, the resonant energies of the two longitudinal modes vary pronouncedly with the intercylinder distance even when the intercylinder distance is about 25 times larger than the cylinder diameter. In contrast, for the transverse modes the splitting of resonant energies becomes apparent when the intercylinder distance falls within about five times of the cylinder diameter. Interestingly, for sufficiently large clusters, each resonance peak contains both magnetic dipole (M1) and electric quadrupole (E2) as well as electric dipole (E1) contributions, and these multipole contributions become rather visible (“bright”) when the distance between the two neighboring cylinders is sufficiently reduced. Finally, the optical plasmon excitation spectra from our simple analytical model are in good qualitative agreement with our DDA calculations.
關聯 J. Physical Chem. C, 114(51), 22398-22405
資料類型 article
dc.contributor 應物所en_US
dc.creator (作者) 郭光宇zh_TW
dc.creator (作者) Klimov, Vasily ; Guo, Guang-Yuen_US
dc.date (日期) 2010.12en_US
dc.date.accessioned 28-Apr-2014 17:42:36 (UTC+8)-
dc.date.available 28-Apr-2014 17:42:36 (UTC+8)-
dc.date.issued (上傳時間) 28-Apr-2014 17:42:36 (UTC+8)-
dc.identifier.uri (URI) http://nccur.lib.nccu.edu.tw/handle/140.119/65647-
dc.description.abstract (摘要) Plasmonic excitations in a three interacting nanocylinder cluster have been investigated by both simple analytical modeling and discrete dipole approximation (DDA) calculations. In our analytical model, each cylinder is regarded as an anisotropic electric dipole with four parameters determined by fitting its optical extinction and scattering spectra to that of DDA simulation. Diagonalization of our analytical model for the three interacting dipoles reveals 10 significant plasmon modes, namely, 5 bright modes and 5 dark eigen-modes. Because of rather long-range longitudinal plasmon coupling, the resonant energies of the two longitudinal modes vary pronouncedly with the intercylinder distance even when the intercylinder distance is about 25 times larger than the cylinder diameter. In contrast, for the transverse modes the splitting of resonant energies becomes apparent when the intercylinder distance falls within about five times of the cylinder diameter. Interestingly, for sufficiently large clusters, each resonance peak contains both magnetic dipole (M1) and electric quadrupole (E2) as well as electric dipole (E1) contributions, and these multipole contributions become rather visible (“bright”) when the distance between the two neighboring cylinders is sufficiently reduced. Finally, the optical plasmon excitation spectra from our simple analytical model are in good qualitative agreement with our DDA calculations.en_US
dc.format.extent 109 bytes-
dc.format.mimetype text/html-
dc.language.iso en_US-
dc.relation (關聯) J. Physical Chem. C, 114(51), 22398-22405en_US
dc.title (題名) Bright and Dark Plasmon Modes in Three Nanocylinder Clusteren_US
dc.type (資料類型) articleen